Spin-phonon coupling and dielectric spectroscopy in nano-crystalline Pr<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline" id="d1e978" altimg="si109.svg"><mml:msub><mml:mrow /><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:math>CoMnO<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline" id="d1e986" altimg="si110.svg"><mml:msub><mml:mrow /><mml:mrow><mml:mn>6</mml:mn></mml:mrow></mml:msub></mml:math> double perovskite manganite

نویسندگان

چکیده

In this paper, we present the spin-phonon coupling and dielectric response of nano-crystalline Pr$_2$CoMnO$_6$ employing Raman spectroscopic study. is a manganite compound , it undergoes paramagnetic to ferromagnetic (PM-FM) phase transition around $T_c$ $\sim$172 K. Temperature-dependent scattering experiment carried out across study behavior in material. The results from reveal an obvious softening phonon mode involving stretching vibrations (Co/Mn)O$_6$ octahedra temperature regions, indicating close correlation between magnetism lattice conform spin coupling. Further, have detailed on response, impedance spectroscopy, electric modulus AC conductivity ceramics range 20 K - 300 frequency 1kHz 5.5MHz. We found shows strong dependence with large dispersion constant. It that thermally activated relaxation mechanism involve material deviated Debye's model which confirmed by Nyquist plot complex modules behavior.

برای دانلود باید عضویت طلایی داشته باشید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Electron-phonon coupling in crystalline pentacene films.

The electron-phonon (e-p) interaction in pentacene (Pn) films grown on Bi(001) was investigated using photoemission spectroscopy. The spectra reveal thermal broadening from which we determine an e-p mass enhancement factor of lambda=0.36+/-0.05 and an effective Einstein energy of omega{E}=11+/-4 meV. From omega{E} it is inferred that dominant contributions to the e-p effects observed in angle-r...

متن کامل

Spin-phonon coupling in antiferromagnetic nickel oxide

E. Aytan, B. Debnath, F. Kargar, Y. Barlas, M. M. Lacerda, J. X. Li, R. K. Lake, J. Shi, and A. A. Balandin Nano-Device Laboratory (NDL), Department of Electrical and Computer Engineering, University of California, Riverside, California 92521, USA Phonon Optimized Engineered Materials (POEM) Center, Materials Science and Engineering Program, University of California, Riverside, California 92521...

متن کامل

Spin-phonon coupling in antiferromagnetic chromium spinels

The temperature dependence of eigenfrequencies and intensities of the IR active modes has been investigated for the antiferromagnetic chromium spinel compounds CdCr2O4, ZnCr2O4, ZnCr2S4, ZnCr2Se4, and HgCr2S4 by IR spectroscopy for temperatures from 5 K to 300 K. At the transition into the magnetically ordered phases, and driven by spin-phonon coupling, most compounds reveal significant splitti...

متن کامل

Strong Carrier–Phonon Coupling in Lead Halide Perovskite Nanocrystals

We highlight the importance of carrier-phonon coupling in inorganic lead halide perovskite nanocrystals. The low-temperature photoluminescence (PL) spectrum of CsPbBr3 has been investigated under a nonresonant and a nonstandard, quasi-resonant excitation scheme, and phonon replicas of the main PL band have been identified as due to the Fröhlich interaction. The energy of longitudinal optical (L...

متن کامل

Heat Transport in Spin Chains with Weak Spin-Phonon Coupling.

The heat transport in a system of S=1/2 large-J Heisenberg spin chains, describing closely Sr(2)CuO(3) and SrCuO(2) cuprates, is studied theoretically at T≪J by considering interactions of the bosonized spin excitations with optical phonons and defects. Treating rigorously the multiboson processes, we derive a microscopic spin-phonon scattering rate that adheres to an intuitive picture of phono...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: Physica B-condensed Matter

سال: 2021

ISSN: ['1873-2135', '0921-4526']

DOI: https://doi.org/10.1016/j.physb.2021.412943